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Crossover from Conventional to Unconventional Superconductivity in 2M-WS2


Abstract Leveraging the reciprocal-space proximity effect between superconducting bulk and topological surface states (TSSs) offers a promising way to topological superconductivity. However, elucidating the mutual influence of bulk and TSSs on topological superconductivity remains a challenge. Here, we report pioneering transport evidence of a thickness-dependent transition from conventional to unconventional superconductivity in 2M-phase WS2 (2M-WS2). As the sample thickness reduces, we see clear changes in key superconducting metrics, including critical temperature, critical current, and carrier density. Notably, while thick 2M-WS2 samples show conventional superconductivity, with an in-plane (IP) upper critical field constrained by the Pauli limit, samples under 20 nm exhibit a pronounced IP critical field enhancement, inversely correlated with 2D carrier density. This marks a distinct crossover to unconventional superconductivity with strong spin-orbit-parity coupling. Our findings underscore the crucial role of sample thickness in accessing topological states in 2D topological superconductors, offering pivotal insights into future studies of topological superconductivity.
Authors Piumi Samarawickrama University of Wyoming , Joseph McBride University of Wyoming , Sabin Gautam University of Wyoming , Zhuangen Fu University of WyomingORCID , Kenji Watanabe ORCID , Takashi Taniguchi ORCID , Wenyong Wang University of Wyoming , Jinke Tang University of WyomingORCID , John Ackerman University of Wyoming , Brian M. Leonard University of WyomingORCID , Jifa Tian University of WyomingORCID
Journal Info American Chemical Society | Nano Letters
Publication Date 12/5/2024
ISSN 1530-6984
TypeKeyword Image article
Open Access closed Closed Access
DOI https://doi.org/10.1021/acs.nanolett.4c05257
KeywordsKeyword Image